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Within the 10.0.7 PTR, it appears this Ensemble is 3 pieces of original 5 piece Paragons of Power Zul'Gurub set Demoniac's Threads

Zandalar Demoniac's Wraps Previously granted when reaching Friendly with the Zandalar Tribe via Paragons of Power: The Demoniac's Wraps
Zandalar Demoniac's Mantle Previously granted when reaching Honored with the Zandalar Tribe via Paragons of Power: The Demoniac's Mantle
Zandalar Demoniac's Robe Previously granted when reaching Revered with the Zandalar Tribe via Paragons of Power: The Demoniac's Robes

As the other two items are not transmoggable, it appears they are not included in the set.

Bought from Rin'wosho il Commerciante in Zul'Grurub after finishing Bijou Ripristinato degli Hakkari for Reliquie di un impero caduto.

He will sell these ensembles in exchange for Emblema per Negoziazioni degli Zandalari and Hakkari bijous of different quality:

As well as the following old Zandalar crafting recipes:

You can get the Emblema per Negoziazioni degli Zandalari and bijous only after completing the quest and achievement.

Emblema per Negoziazioni degli Zandalari can be obtained from Rin'wosho inside of the Zul'Gurub dungeon, in exchange for various troll coins.
You'll need at least one of each from the following sets before he'll offer a repeatable quest to exchange them:

Moneta Zuliana + Moneta Razzashi + Moneta degli Hakkari
Moneta Sabbiafurente + Moneta Fendicranio + Moneta Scalporosso
Moneta dei Gurubashi + Moneta Ramovile + Moneta Scorzasecca

Coins have a chance to drop from trolls inside the Zul'gurub Heroic Dungeon after earning Reliquie di un impero caduto.
They can also be fished directly from the waters in the dungeon, or from caches like Sacchettino per Una Monetina dei Modelli, which can also be fished from the waters.
Lastly they're purchasable from the Auction House, and appear to be a Region-Wide Commodity.

Riassunto

Screenshot

Video

Set: Demoniaco degli Zandalari

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[This item can be purchased in] Dazar'alor (2) e Zul'gurub .